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To understand the low-energy structure of the neutron deficient iodine isotopes, lifetimes for the low-lying 9/2+ and 11/2+ positive-parity states in 113I have been measured as τ = 28(4) ps and τ = 3.7(7) ps, respectively. The lifetime for the 11/2− state, which feeds the 9/2+ and 11/2+ states, was remeasured with improved accuracy as τ = 216(7) ps. The reduced transition probability, B(E2) = 32(5) W.u., for the 9/2+ → 5/2+ transition agrees with that calculated within the shell model using a Hamiltonian based on the charge-dependent Bonn nucleon-nucleon interaction. In contrast, the much larger transition probability, B(E2) = 209(39) W.u., measured for the 11/2+ → 7/2+ transition has been interpreted, with the aid of configuration-constrained total Routhian surface calculations, as resulting from a slightly γ -soft rotor with an associated quadrupole deformation of β2 ≈ 0.18. Remarkably similar reduced E1 transition probabilities of 5.5(5) × 10−4 and 4.9(5) × 10−4 W.u. were deduced for the 11/2− → 9/2+ and 11/2− → 11/2+ transitions, respectively, which feed apparently dissimilar but competing structures.
The 278-keV M2 γ decay from the νh11/2 isomeric state in 113Xe has been observed for the first time using the recoil-isomer tagging technique. The half-life of the isomer has been measured to be 6.9(3) μs. The derived B(M2) value is in agreement with the trend of systematic measurements of M2 transition strengths in neutron-deficient tellurium and tin isotopes. The lifetime of the first excited state in the νh11/2 band has been measured using the recoil distance Doppler-shift method. The extracted B(E2) value has been compared to theoretical CD-Bonn calculations and recent lifetime measurements in 109Te. This comparison of B(E2) values has been used to shed light on the possible influence of collective degrees of freedom on M2 transition strengths in the most neutron-deficient xenon nuclei. The νh11/2 band is deduced to have a degree of deformation comparable with the ground-state bands of the even-mass xenon isotopes. However, the value deduced in this work indicates a loss of collective behavior when compared with the lower-mass 109Te. This result suggests that, while changes in deformation may be partly responsible for the observed trend in B(M2) values for increasing Z, other effects may also be present.
Lifetime measurements have been made in the neutron-deficient nucleus 109Te using the coincident recoil distance Doppler-shift method. The experimental B(E2) values have been compared with state-of-the-art shellmodel calculations using the monopole-corrected realistic charge-dependent Bonn nucleon-nucleon potential. Lifetimes in the νh11/2 band are consistent with an interpretation based on the deformation driving properties of a single valence neutron outside of the even-even tellurium core and highlight the unexpected presence of collective behavior as the N = 50 shell closure is approached. Lifetime measurements for the low-lying positive-parity states also appear to correlate well with shell-model calculations. In addition, a comparison with the proton-unbound nucleus 109I suggests that the presence of a single decoupled valence proton affects the total measured B(E2) strengths in a manner that is not currently well understood.
Lifetimes of low-lying excited states in the νi13/2+ bands of the neutron-deficient osmium isotopes 169,171,173Os have been measured for the first time using the recoil-distance Doppler shift and recoil-isomer tagging techniques. An unusually low value is observed for the ratio B(E2; 21/2+ →17/2+)/B(E2; 17/2+ → 13/2+) in 169Os, similar to the “anomalously” low values of the ratio B(E2; 41+ → 21+)/B(E2; 21+ → 0+gs) previously observed in several transitional rare-earth nuclides with even numbers of neutrons and protons, including the neighbouring 168,170Os. Furthermore, the evolution of B(E2; 21/2+ → 17/2+)/B(E2; 17/2+ → 13/2+) with increasing neutron number in the odd-mass isotopic chain 169,171,173Os is observed to follow the same trend as observed previously in the even-even Os isotopes. These findings indicate that the possible quantum phase transition from a seniority conserving structure to a collective regime as a function of neutron number suggested for the even-even systems is maintained in these odd-mass osmium nuclei, with the odd valence neutron merely acting as a “spectator”. As for the even-even nuclei, the phenomenon is highly unexpected for nuclei that are not situated near closed shells.
Lifetimes of the first excited 2 + and 4 + states in the extremely neutron-deficient nuclide 172 Pt have been measured for the first time using the recoil-distance Doppler shift and recoil-decay tagging techniques. An unusually low value of the ratio B ( E 2 : 4 + 1 → 2 + 1 ) / B ( E 2 : 2 + 1 → 0 + gs ) = 0.55 ( 19 ) was found, similar to a handful of other such anomalous cases observed in the entire Segré chart. The observation adds to a cluster of a few extremely neutron-deficient nuclides of the heavy transition metals with neutron numbers N ≈ 90 – 94 featuring the effect. No theoretical model calculations reported to date have been able to explain the anomalously low B ( E 2 : 4 + 1 → 2 + 1 ) / B ( E 2 : 2 + 1 → 0 + gs ) ratios observed in these cases. Such low values cannot, e.g., be explained within the framework of the geometrical collective model or by algebraic approaches within the interacting boson model framework. It is proposed that the group of B ( E 2 : 4 + 1 → 2 + 1 ) / B ( E 2 : 2 + 1 → 0 + gs ) ratios in the extremely neutron-deficient even-even W, Os, and Pt nuclei around neutron numbers N ≈ 90 – 94 reveal a quantum phase transition from a seniority-conserving structure to a collective regime as a function of neutron number. Although a system governed by seniority symmetry is the only theoretical framework for which such an effect may naturally occur, the phenomenon is highly unexpected for these nuclei that are not situated near closed shells.
Excited states in the extremely neutron-deficient nucleus 172Pt were populated via 96Ru(78Kr, 2p) and 92Mo(83Kr, 3n) reactions. The level scheme has been extended up to an excitation energy of ≈ 5 MeV and tentative spin-parity assignments up to I π = 18+. Linear polarization and angular distribution measurements were used to determine the electromagnetic E1 character of the dipole transitions connecting the positive-parity ground-state band with an excited side-band, firmly establishing it as a negativeparity band. The lowest member of this negative-parity structure was firmly assigned spin-parity 3−. In addition, we observed an E3 transition from this 3− state to the ground state, providing direct evidence for octupole collectivity in 172Pt. Large-scale shell model (LSSM) and total Routhian surface (TRS) calculations have been performed, supporting the interpretation of the 3− state as a collective octupolevibrational state.
Abstract Lifetimes of low-lying excited states in the vi13/2+ bands of the neutron-deficient osmium isotopes 169,171,173Os have been measured for the first time using the recoil-distance Doppler shift and recoil-isomer tagging techniques. An unusually low value is observed for the ratio B(E2; 21/2+ → 17/2+) /B(E2; 17/2+ → 13/2+) in 169Os, similar to the “anomalously” low values of the ratio B(E2; 4+1 → 2+1 )/B(E2; 2+1 → 0+gs) previously observed in several transitional rare-earth nuclides with even numbers of neutrons and protons, including the neighboring 168,170Os. Furthermore, the evolution of B(E2; 21/2+→ 17/2+)/B(E2; 17/2+ → 13/2+) with increasing neutron number in the odd-mass isotopic chain 169,171,173Os is observed to follow the same trend as observed previously in the even-even Os isotopes. These findings indicate that the possible quantum phase transition from a seniority conserving structure to a collective regime as a function of neutron number suggested for the even-even systems is maintained in these odd-mass osmium nuclei, with the odd valence neutron merely acting as a “spectator”. As for the even-even nuclei, the phenomenon is highly unexpected for nuclei that are not situated near closed shells.