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One new pair of positive-parity chiral doublet bands have been identified in the odd-A nucleus 135Nd which together with the previously reported negative-parity chiral doublet bands constitute a third case of multiple chiral doublet (MχD) bands in the A ≈ 130 mass region. The properties of the MχD bands are well reproduced by constrained covariant density functional theory and particle rotor model calculations. The newly observed MχD bands in 135Nd represents an important milestone in supporting the existence of MχD in nuclei.
Abstract One new pair of positive-parity chiral doublet bands have been identified in the odd-A nucleus 135Nd which together with the previously reported negative-parity chiral doublet bands constitute a third case of multiple chiral doublet (MχD) bands in the A≈130 mass region. The properties of the MχD bands are well reproduced by constrained covariant density functional theory and particle rotor model calculations. The newly observed MχD bands in 135Nd represents an important milestone in supporting the existence of MχD in nuclei.
Abstract Two new excited bands built on the πh11/2 configuration have been identified in 135Nd in addition to the known πh11/2 band. The energy spectra of the excited bands and the available electromagnetic transition probabilities are in good agreement with theoretical results obtained using quasiparticle-plus-triaxial-rotor model calculations. The properties of the bands identify them as tilted precession bands instead of wobbling bands. Our results give a new insight into the interpretation of the low-lying bands in odd-A mass nuclei, and can stimulate future studies to address the nuclear triaxiality.
Abstract The nature of two high-spin bands in 136 built on the two-quasiparticle configuration πh211/2, predicted by the triaxial projected shell model as good candidates of transverse wobbling bands, are investigated experimentally. The mixing ratio of one ΔI=1 transition connecting the one-phonon and the zero-phonon wobbling bands is established from a high-statistics JuroGam II γ-ray spectroscopy experiment by using the combined angular correlation and linear polarization method. The resulting wobbling excitation energy and ratios of reduced electromagnetic transition probabilities are in good agreement with results of a new particle-rotor model which rigidly couples the total angular momentum of two quasiparticles to a triaxial core in an orthogonal geometry, confirming thus the transverse wobbling nature of the bands.
Abstract The electromagnetic character of the ΔI = 1 transitions connecting the 1- to 0-phonon and the 2- to 1-phonon wobbling bands should be dominated by an E2 component, due to the collective motion of the entire nuclear charge. In the present work it is shown, based on combined angular correlation and linear polarization measurements, that the mixing ratios of all analyzed connecting transitions between low-lying bands in 135Pr interpreted as 0-, 1-, and 2-phonon wobbling bands, have absolute values smaller than one. This indicates predominant M1 magnetic character, which is incompatible with the proposed wobbling nature. All experimental observables are instead in good agreement with quasiparticle-plus-triaxial-rotor model calculations, which describe the bands as resulting from a rapid re-alignment of the total angular momentum from the short to the intermediate nuclear axis.
Abstract Experimental signatures of moderately enhanced octupole correlations at high spin in 136Nd are indicated for the first time. The extracted dipole moments of two negative-parity bands are only two times smaller than those of the lanthanide nuclei with N≈90 which present well-established octupole correlations. Calculations using the cranked quasiparticle random phase approximation and a model of quadrupole-octupole rotations with octupole vibrations reveal the structure of the bands and the enhanced octupole correlations at high spin in 136Nd.
Two new excited bands built on the πh11/2 configuration have been identified in 135Nd in addition to the known πh11/2 band. The energy spectra of the excited bands and the available electromagnetic transition probabilities are in good agreement with theoretical results obtained using quasiparticle-plus-triaxial-rotor model calculations. The properties of the bands identify them as tilted precession bands instead of wobbling bands. Our results give a new insight into the interpretation of the low-lying bands in odd-A mass nuclei, and can stimulate future studies to address the nuclear triaxiality.
The nature of two high-spin bands in 136Nd built on the two-quasiparticle configuration πh211/2, predicted by the triaxial projected shell model as good candidates of transverse wobbling bands, are investigated experimentally. The mixing ratio of one ΔI=1 transition connecting the one-phonon and the zero-phonon wobbling bands is established from a high-statistics JuroGam II γ-ray spectroscopy experiment by using the combined angular correlation and linear polarization method. The resulting wobbling excitation energy and ratios of reduced electromagnetic transition probabilities are in good agreement with results of a new particle-rotor model which rigidly couples the total angular momentum of two quasiparticles to a triaxial core in an orthogonal geometry, confirming thus the transverse wobbling nature of the bands.
The electromagnetic character of the ΔI=1 transitions connecting the 1- to 0-phonon and the 2- to 1-phonon wobbling bands should be dominated by an E2 component, due to the collective motion of the entire nuclear charge. In the present work it is shown, based on combined angular correlation and linear polarization measurements, that the mixing ratios of all analyzed connecting transitions between low-lying bands in 135Pr interpreted as 0-, 1-, and 2-phonon wobbling bands, have absolute values smaller than one. This indicates predominant M1 magnetic character, which is incompatible with the proposed wobbling nature. All experimental observables are instead in good agreement with quasiparticle-plus-triaxial-rotor model calculations, which describe the bands as resulting from a rapid re-alignment of the total angular momentum from the short to the intermediate nuclear axis.
Abstract The level structure of 136Nd has been investigated using the 100Mo(40Ar, 4n) reaction and the JUROGAM II+RITU+GREAT setup. The level scheme has been extended significantly. Many new bands have been identified both at low and high spin, among which are five nearly degenerate bands interpreted as chiral partners. Excitation energies, spins, and parities of the previously known bands are revised and firmly established, and some previously known bands have been revised. Configurations are assigned to the observed bands based on cranked Nilsson-Strutinsky calculations. The band structure of 136Nd is now clarified and the various types of single-particle and collective excitations are well understood.
Experimental signatures of moderately enhanced octupole correlations at high spin in 136Nd are indicated for the first time. The extracted dipole moments of two negative-parity bands are only two times smaller than those of the lanthanide nuclei with N≈90 which present well-established octupole correlations. Calculations using the cranked quasiparticle random phase approximation and a model of quadrupole-octupole rotations with octupole vibrations reveal the structure of the bands and the enhanced octupole correlations at high spin in 136Nd.
Three new highly-deformed (HD) bands are identified in 136Nd and the highly deformed band of 137Nd is extended at higher spin by four transitions, revealing a band crossing associated with the occupation of the second νi13/2 intruder orbital. Extended cranked Nilsson-Strutinsky calculations are performed for all HD bands observed in 134Nd, 136Nd, and 137Nd, achieving for the first time a consistent interpretation of all HD bands in the Nd nuclei. The new interpretation has significant consequences, like the change of parity of the yrast HD bands of 134Nd and 136Nd, and the involvement of two negative-parity neutron intruder orbitals in the configurations of most HD bands. The present experimental results and their theoretical interpretation represent an important step forward in the understanding of the second-minimum excitations in the Nd nuclei.
The neutron-deficient 119Ba nucleus has been studied using the 58Ni(64Zn,2pn) reaction and the JUROGAM 3 γ-ray detector array coupled to the MARA recoil-mass separator setup. One new rotational band and several low-lying states are newly identified. A half-life of T1/2=0.36(2)μs has been measured for the 5/2− bandhead of the νh11/2 band. The two previously known rotational bands are confirmed, except for the higher part of the +1/2 signature partner of the positive-parity band. Configurations are assigned based on the analysis of the observed quasiparticle alignments whose nature is unveiled by the calculations using the particle number conserving cranked shell model.
One of the largest sets of collective excitations built on two-quasiparticle configurations in odd-odd nuclei of the proton-rich A≈120 mass region is reported in 118Cs. Several new rotational bands and long-lived isomers have been identified. The 8+ bandhead of the πh11/2⊗νh11/2 band is a short-lived isomer with a half-life in the nanosecond range, while the 7+ state below it is a long-lived isomer with a half-life of T1/2=0.55(6)μs. Two other long-lived isomers have been identified: a 66-keV transition detected at the MARA focal plane depopulates one of them, indicating a half-life in the microsecond range, while no depopulating transitions have been identified for the other, indicating a much longer half-life. Extensive particle number conserving cranked shell model calculations and alignment analysis have been employed to investigate the rich band structure of 118Cs, which exhibits one of the most complete sets of two-quasiparticle configurations in nuclei close to the proton drip line.
The very neutron-deficient strongly deformed 119Cs nucleus has been studied using the 58Ni(64Zn,3p) reaction and the JUROGAM 3 γ-ray detector array coupled to the MARA recoil-mass separator setup. The excitation energies of all observed bands have been determined, spins and parities have been firmly assigned to most of the observed states. The previously known and the newly identified rotational bands have been extended to very high spin and excitation energy. The configurations of the observed bands are discussed using the particle number conserving cranked shell model. The present study establishes the largest set of rotational bands observed in the proton-rich A≈120 mass region.
Prolate-oblate shape coexistence close to the ground state in the strongly-deformed proton-rich A≈120 nuclei is reported for the first time. One of the four reported bands in 119Cs, built on a 11/2− state at 670 keV, consists of nearly degenerate signature partners, and has properties which unequivocally indicate the strongly-coupled πh11/2[505]11/2− configuration associated with oblate shape. Together with the decoupled πh11/2[541]3/2− band built on the 11/2− prolate state at 110 keV, for which a half-life of T1/2=55(5)μs has been measured, the new bands bring evidence of shape coexistence at low spin in the proton-rich strongly deformed A≈120 nuclei, a phenomenon predicted since long time, but not yet observed. Calculations using the particle-number conserving cranked shell model and two dimensional tilted axis cranking covariant density functional theory support and well reproduce the observed oblate and prolate coexisting low-energy states in 119Cs.
Three new negative-parity bands have been identified in 120Ba, two of them forming a strongly coupled band. The previously known negative-parity band is significantly extended to high spin, while the lower part of the yrare positive-parity band has been modified. From the analysis of the band properties and comparison with the neighboring nuclei a coherent description of all bands is achieved. In particular, a simple explanation of the evolution of the positive-parity bands at high spin is proposed, including the possible occupation of the νf7/2[541]1/2− intruder orbital. Cranked Nilsson-Strutinsky calculations reveal similar quadrupole deformations but different triaxiality of the bands, while particle number conserving cranked shell model calculations qualitatively reproduce the experimental data and support the assigned configurations. The new measured ratios of reduced transition probabilities B(E1)/B(E2) complete the systematics in the 118–124Ba nuclei, exhibiting a decrease with decreasing neutron number, and are compared with the known values in the 116–120Xe nuclei, which are larger. Extended calculations with the quadrupole and octupole collective Hamiltonian based on the relativistic Hartree-Bogoliubov model employing the relativistic DD-PC1 density functional nicely reproduce the decreasing trend towards lower neutron numbers for Ba and Xe nuclei, as well as the larger values in Xe nuclei, but are much larger in amplitude than the experimental values. On the other hand, particle number conserving cranked shell model calculations without octupole deformation overestimate the low-spin values, while those with octupole deformation included reproduce the experimental values in 120Ba, suggesting the possible existence of moderate octupole collectivity in the negative-parity bands of nuclei in this mass region.
Knowledge of the exact microscopic structure of the 01 + ground state and first excited 02 + state in 150Sm is required to understand the branching of double β decay to these states from 150Nd. The detailed spectroscopy of 150Sm and 152Gd has been studied using (α,xn) reactions and the γ -ray arrays AFRODITE and JUROGAM II. Consistently strong E1 transitions are observed between the excited Kπ = 02 + bands and the lowest negative parity bands in both nuclei. These results are discussed in terms of the possible permanent octupole deformation in the first excited Kπ = 02 + band and also in terms of the “tidal wave” model of Frauendorf.
Linear polarization measurements have been performed for γ rays in 91Ru produced with the 58Ni(36Ar, 2p1nγ ) 91Ru reaction at a beam energy of 111 MeV. The EXOGAM Ge clover array has been used to measure the γ -γ coincidences, γ -ray linear polarization, and γ -ray angular distributions. The polarization sensitivity of the EXOGAM clover detectors acting as Compton polarimeters has been determined in the energy range 0.3–1.3 MeV. Several transitions have been observed for the first time. Measurements of linear polarization and angular distribution have led to the firm assignments of spin differences and parity of high-spin states in 91Ru. More specifically, calculations using a semiempirical shell model were performed to understand the structures of the first and second (21/2+) and (17/2+) levels. The results are in good agreement with the experimental data, supporting the interpretation of the nonyrast (21/2+) and (17/2+) states in terms of the Jmax and Jmax − 2 members of the seniority-three ν(g9/2) −3 multiplet.
Low-spin states of 157Dy have been studied using the JUROGAM II array, following the 155Gd (α, 2n) reaction at a beam energy of 25 MeV. The level scheme of 157Dy has been expanded with four new bands. Rotational structures built on the [523]5/2− and [402]3/2+ neutron orbitals constitute new additions to the level scheme as do many of the inter- and intraband transitions. This manuscript also reports the observation of cross I+→(I–1)− and I−→(I–1)+ E1 dipole transitions interlinking structures built on the [523]5/2− (band 5) and [402]3/2+ (band 7) neutron orbitals. These interlacing band structures are interpreted as the bands of parity doublets with simplex quantum number s=–i related to possible octupole correlations.
A sequence of nine almost equidistant quadrupole transitions is observed in 137Nd. The sequence represents an extremely regular rotational band that extends to a spin of about 75/2 and an excitation energy of ≈4.5 MeV above yrast. Cranked mean-field calculations of the Nilsson-Strutinsky type suggest an oblate shape for the band. They reproduce the observed I(I + 1) dependence of the rotational energy whereas predicting a pronounced decrease in the deformation, which is the hallmark of antimagnetic rotation.
Doppler Shift Attenuation Method (DSAM) analysis of excited-state lifetimes normally employs thin production targets mounted on a thick stopper foil (“backing”) serving to slow down and stop the recoiling nuclei of interest in a well-defined manner. Use of a thick, homogeneous production target leads to a more complex analysis as it results in a substantial decrease in the energy of the incident projectile which traverses the target with an associated change in the production cross section of the residues as a function of penetration depth. Here, a DSAM lifetime analysis using a thick homogeneous target has been verified using the Doppler broadened lineshapes of γ rays following the decay of highly excited states in the semi-magic (N = 50) nucleus 94Ru. Lifetimes of excited states in the 94Ru nucleus have been obtained using a modified version of the LINESHAPE package from the Doppler broadened lineshapes resulting from the emission of the γ rays, while the residual nuclei were slowing down in the thick (6 mg/cm2 ) metallic 58Ni target. The results have been validated by comparison with a previous measurement using a different (RDDS) technique.
The level structure of 136Nd has been investigated using the 100Mo(40Ar, 4n) reaction and the JUROGAM II+RITU+GREAT setup. The level scheme has been extended significantly. Many new bands have been identified both at low and high spin, among which are five nearly degenerate bands interpreted as chiral partners. Excitation energies, spins, and parities of the previously known bands are revised and firmly established, and some previously known bands have been revised. Configurations are assigned to the observed bands based on cranked Nilsson-Strutinsky calculations. The band structure of 136Nd is now clarified and the various types of single-particle and collective excitations are well understood.
A comprehensive systematic study is made for the collective β and γ bands in even-even isotopes with neutron numbers N=88 to 92 and proton numbers Z=62(Sm) to 70 (Yb). Data, including excitation energies, B(E0) and B(E2) values, and branching ratios from previously published experiments are collated with new data presented for the first time in this study. The experimental data are compared to calculations using a five-dimensional collective Hamiltonian (5DCH) based on the covariant density functional theory (CDFT). A realistic potential in the quadrupole shape parameters V(β,γ) is determined from potential energy surfaces (PES) calculated using the CDFT. The parameters of the 5DCH are fixed and contained within the CDFT. Overall, a satisfactory agreement is found between the data and the calculations. In line with the energy staggering S(I) of the levels in the 2γ+ bands, the potential energy surfaces of the CDFT calculations indicate γ-soft shapes in the N=88 nuclides, which become γ rigid for N=90 and N=92. The nature of the 02+ bands changes with atomic number. In the isotopes of Sm to Dy, they can be understood as β vibrations, but in the Er and Yb isotopes the 02+ bands have wave functions with large components in a triaxial superdeformed minimum. In the vicinity of 152Sm, the present calculations predict a soft potential in the β direction but do not find two coexisting minima. This is reminiscent of 152Sm exhibiting an X(5) behavior. The model also predicts that the 03+ bands are of two-phonon nature, having an energy twice that of the 02+ band. This is in contradiction with the data and implies that other excitation modes must be invoked to explain their origin.
Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C,5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-A155,157Dy isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei 154Dy and 156Dy are also discussed.
Lifetimes of negative-parity states have been determined in the neutron deficient semi-magic (N = 50) nucleus 95Rh. The fusion-evaporation reaction 58Ni(40Ca,3p) was used to populate high-spin states in 95Rh at the Grand Accélérateur National d’Ions Lourds (GANIL) accelerator facility. The results were obtained using the Doppler Shift Attenuation Method (DSAM) based on the Doppler broadened line shapes produced during the slowing down process of the residual nuclei in a thick 6mg/cm2 metallic target. B(M1) and B(E2) reduced transition strengths are compared with predictions from large-scale shell-model calculations.
Abstract Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C,5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-A155,157Dy isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei 154Dy and 156Dy are also discussed.
Evidence for chiral doublet bands has been observed for the first time in the even-even nucleus 136 Nd . One chiral band was firmly established. Four other candidates for chiral bands were also identified, which can contribute to the realization of the multiple pairs of chiral doublet bands ( M χ D ) phenomenon. The observed bands are investigated by the constrained and tilted axis cranking covariant density functional theory (TAC-CDFT). Possible configurations have been explored. The experimental energy spectra, angular momenta, and B ( M 1 ) / B ( E 2 ) values for the assigned configurations are globally reproduced by TAC-CDFT. Calculated results support the chiral interpretation of the observed bands, which correspond to shapes with maximum triaxiality induced by different multiquasiparticle configurations in 136 Nd .